Atomic and Molecular Processes with Short Intense Laser Pulses

Atomic and Molecular Processes with Short Intense Laser Pulses PDF

Author: Andre D. Bandruk

Publisher: Springer Science & Business Media

Published: 2012-12-06

Total Pages: 460

ISBN-13: 1461309670

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This volume contains the lectures and communications presented at the NATO Advanced Research Workshop on "Atomic and Molecular Processes with Short Intense Laser Pulses" (NATO ARW 848/86). The workshop was held at Bishop's University, Lennoxville, Que, Canada, July 19-24, 1987, under the directorship of Prof. A.D. Bandrauk, Universite de Sherbrooke. A scientific committee made up of Dr. P. Corkum (Laser Physics, ~ational Research Council of Canada), Dr. P. Hackett (Laser Chemistry, National Research Council of Canada), Prof. S.C. Wallace (Dept. of Chemistry and Physics, University of Toronto), and Prof. F.H.M. Faisal (FakultHt fUr Physik, UniversitHt Bellefeld) was called upon to invite and organize eminent lectures in the fields of i) Coherence Phenomena in Atomic and Molecular Photoprocesses. ii) High Intensity Atomic and Molecular Phenomena. iii) Laser Chemistry The aim of the workshop was to bring together chemists and physicists in order to~iscuss and analyze the progress made in the use of short in tense laser pulses in understanding coherence phenomena and high intensity, nonlin~adiative effects in atomic and molecular systems.

Super-Intense Laser—Atom Physics

Super-Intense Laser—Atom Physics PDF

Author: A. L'Huillier

Publisher: Springer Science & Business Media

Published: 2012-12-06

Total Pages: 494

ISBN-13: 1461579635

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The rapid development of powerful pulsed lasers is at the origin of a conside rable interest in studying the response of an atom, a molecule (or a solid) to a strong electromagnetic field. It is now possible to produce at the laboratory scale, ultra-short 13 pulses with a duration of 100 femtoseconds (10- second) and a power of the order 12 of 1 terawatt (10 Watt). Under these conditions, very high peak intensities may be obtained and electric fields exceeding typical electron binding fields in atoms are generated. The interaction of an atom or a molecule with such electromagnetic fields has a highly non-linear character which leads to unexpected phenomena. Amongst them, - above-threshold ionization (ATI) i.e. the absorption of additional photons in excess of the minimal number necessary to overcome the ionization potential and its molecular counterpart, above-threshold dissociation (ATD); - generation of very high harmonics of the driving field; - stabilization of one-electron systems in strong fields. These processes were the main topics of two international meetings which were held in 1989 and 1991 in the United States under the common name SILAP (Super-Intense Laser-Atom Physics).

Super-Intense Laser-Atom Physics

Super-Intense Laser-Atom Physics PDF

Author: Bernard Piraux

Publisher: Springer

Published: 2001-03-31

Total Pages: 416

ISBN-13: 9780792368632

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The study of atomic systems exposed to super-intense laser fields de fines an important area in atomic, molecular and optical physics. Although the concept of super-intense field has no absolute meaning, it is now usual to call an electromagnetic field super-intense when it exceeds the atomic binding field. In the case of the simplest atomic system, hydrogen in its 16 2 ground state, this occurs above an intensity of 3. 5 x 10 Wattfcm which is the atomic unit of intensity. Presently at the laboratory scale and in ex tremely short and tightly focussed laser pulses, the electric field strength 16 18 2 reaches peak values which are of the order of 10 - 10 Wattfcm in the infrared frequency regime, the prospect being that such peak intensities may be reached within a few years in a regime of much higher frequencies (XUV or even X). The interaction of such electromagnetic fields with an atomic system has a highly non-linear character which has led to the observation of to tally unexpected phenomena. There are three fundamental processes which have marked the beginning of an intensive research in the field of super intense laser-atom physics (SILAP). These processes which only involve one atomic electron are (i) the so-called above-threshold ionisation i. e.

Coherence Phenomena in Atoms and Molecules in Laser Fields

Coherence Phenomena in Atoms and Molecules in Laser Fields PDF

Author: Andre D Bandrauk

Publisher: Springer Science & Business Media

Published: 2012-12-06

Total Pages: 397

ISBN-13: 1461533643

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This volume contains the lectures and communications presented at the NATO Advanced Research Workshop (NATO ARW 900857) which was held May 5-10, 1991 at McMaster University, Hamilton, Ontario, Canada. A scientific commitee made up of P.P. Lambropoulos (USC & Crete), P.8. Corkum (NRC, Ottawa), and H. B. vL. van den Heuvell (FOM, Amsterdam) guided the organizers, A.D. Bandrauk (Sherbrooke) and S.C. Wallace (Toronto) in preparing a programme which would cover the latest advances in the field of atom and molecule laser interactions. Since the last meeting held in July 1987 on "Atomic and Molecular Processes with Short Intense Laser Pulses", NATO ASI vol 1718 (Plenum Press 1988), considerable progress has been made in understanding high intensity effects on atoms and the concomitant coherence effects. After four years, the emphasis is now shifting more to molecules. The present volume represents therefore this trend with four sections covering the main interests of research endeavours in this area: i) Atoms in Intense Laser-Fields ii) Molecules in Intense Laser Fields iii) Atomic Coherences iv) Molecular Coherences The experience developed over the years in multiphoton atomic processes has been very useful and is the main source of our understanding of similar processes in molecules. Thus ATI (above threshold ionization) has been found to occur in molecules as well as a new phenomenon, ATD (above-threshold dissociation). Laser-induced avoided crossings of molecular electronic surfaces is also now entering the current language of high intensity molecular processes.

Ultrafast Dynamics Driven by Intense Light Pulses

Ultrafast Dynamics Driven by Intense Light Pulses PDF

Author: Markus Kitzler

Publisher: Springer

Published: 2015-07-24

Total Pages: 385

ISBN-13: 3319201735

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This book documents the recent vivid developments in the research field of ultrashort intense light pulses for probing and controlling ultrafast dynamics. The recent fascinating results in studying and controlling ultrafast dynamics in ever more complicated systems such as (bio-)molecules and structures of meso- to macroscopic sizes on ever shorter time-scales are presented. The book is written by some of the most eminent experimental and theoretical experts in the field. It covers the new groundbreaking research directions that were opened by the availability of new light sources such as fully controlled intense laser fields with durations down to a single oscillation cycle, short-wavelength laser-driven attosecond pulses and intense X-ray pulses from the upcoming free electron lasers. These light sources allowed the investigation of dynamics in atoms, molecules, clusters, on surfaces and very recently also in nanostructures and solids in new regimes of parameters which, in turn, led to the identification of completely new dynamics and methods for controlling it. Example topics covered by this book include the study of ultrafast processes in large molecules using attosecond pulses, control of ultrafast electron dynamics in solids with shaped femtosecond laser pulses, light-driven ultrafast plasmonic processes on surfaces and in nanostructures as well as research on atomic and molecular systems under intense X-ray radiation. This book is equally helpful for people who would like to step into this field (e.g. young researchers), for whom it provides a broad introduction, as well as for already experienced researchers who may enjoy the exhaustive discussion that covers the research on essentially all currently studied objects and with all available ultrafast pulse sources.

Atoms, Solids, and Plasmas in Super-Intense Laser Fields

Atoms, Solids, and Plasmas in Super-Intense Laser Fields PDF

Author: Dimitri Batani

Publisher: Springer Science & Business Media

Published: 2001-09-30

Total Pages: 434

ISBN-13: 9780306466151

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Proceedings of the 30th Course of the International School of Quantum Electronics on Atoms, Solids and Plasmas in Super-Intense Laser Fields, held 8-14 July, in Erice, Sicily

Laser Control of Atoms and Molecules

Laser Control of Atoms and Molecules PDF

Author: Vladilen Letokhov

Publisher: OUP Oxford

Published: 2007-02-15

Total Pages: 328

ISBN-13: 0191523712

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Rather different problems can be lumped together under the general term 'laser control of atoms and molecules'. They include the laser selection of atomic and molecular velocities for the purpose of Doppler-free spectroscopy, laser control of the position and velocity of atoms (i.e. laser trapping and cooling of atoms), and laser control of atomic and molecular processes (ionization, dissociation) with a view of detecting single atoms and molecules and particularly separating isotopes and nuclear isomers. Over the last decades the principal problems posed have been successfully solved, and many of them have evolved remarkably in the subsequent investigations of the international research community. For example, the solution of the problem of laser cooling and trapping of atoms has given birth to the new field of the physics of ultracold matter, i.e. quantum atomic and molecular gases. The laser non-coherent control of uni-molecular processes has found an interesting extension in the field of laser coherent control of molecules. The concept of laser control of position has been successfully demonstrated with microparticles (optical tweezers), concurrently with investigations into atomic control. The laser photo-ionization of molecules on surfaces has led to the development of novel techniques of laser-assisted mass spectrometry of macromolecules, and so on. The aim of this book is to review these topics from a unified or 'coherent' point of view. It will be useful for many readers in various fields of laser science and its applications.

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